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Chloe Smith's work experience begins in 2016 when they co-founded bigmoose coffee co, a company with a mission to improve the world. Their responsibilities included updating social media and organizing events to raise money for charitable causes. In 2016, they also worked on the Pritchard's 100k Challenge, overseeing the social media strategy for a world record challenge. Additionally, Chloe worked as a Hospitality Supervisor for Bespoke Event Team from 2013 until 2023. Currently, Chloe serves as the Chief Operations Officer for bigmoose, a role they started in 2022.

Chloe Smith's education history includes attending Howells School Llandaff from 2006 to 2013. Chloe then went on to study at the University of South Wales, where they earned a Bachelor of Arts Honors degree in Primary Studies. No specific field of study is mentioned for their primary studies degree.