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Ali Mustoe-Playfair has a diverse work experience spanning multiple companies and roles. They started their career in 2006 at Genesis Communications as an Academy Sales Support before transitioning to Sales Operations Executive. In 2008, they joined Outsourcery as a Service Relationship Manager and later became the London Office Manager. From 2018 to 2019, Ali worked at PHYSIOTHERAPY2FIT LTD as an Operations Manager. In 2020, they worked as a Funeral Arranger at Co-operative funeralcare before moving to ANS Group. At ANS Group, they held various positions including Internal Sales Account Manager, Alliances Operations Manager, and PMO Lead. Currently, they are the Head of Business Operations at ANS Group.

Ali Mustoe-Playfair attended Highsted Grammar School from 1995 to 2000. No degree or field of study information is provided. In addition to formal education, Ali Mustoe-Playfair obtained certifications such as "House of PMO - Essentials for PMO Administrators" from APMG International in January 2023 and "Microsoft Certified: Dynamics 365 Fundamentals" from Microsoft in March 2021.